Yeah so you are going to be disappointed. DS hacking is far behind GBA hacking. All you will find are adjusted difficulty/catch-em-all hacks. That being said, for Gen 4, there is Bloody Platinum and Flawless Platinum.
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Both increase difficulty and let you catch all 493 Pokemon up through Gen 4. Drayano makes good hacks too. He has several. Storm Silver and Sacred Gold (I think those are the names) are hacks of Heart Gold and Soul Silver.
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Blaze Black and Volt White are hacks of Black and White. Blaze Black 2 and Volt White 2 are hacks of Black 2 and White 2. All of the above mentioned hacks increase difficulty and let you catch every Pokemon up through that generation. There are 3DS hacks too but there is no working 3DS emulator as far as I know so I don’t play them.
Edit: there is an ongoing project to port the GBA hack “Light Platinum” into DS but last time I checked it wasn’t even close to being done. I can do that. So I’m not going to go into exceptional detail about any of these and they aren’t necessarily in order of quality or enjoyment.
Glazed is definitely the best. Regions (one new full region, a redesigned Johto, and then a smaller 3rd new region). Blazed Glazed is an updated version so I would suggest that.
Light Platinum is another good one. Usually makes Top 10 lists. It’s a bit easier than I prefer though.
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I think Light Platinum + is the most updated version. Flora Sky is a sort of bland hack.
It originally came out in like 2011 but there is a more updated version. It’s a full new region with some post-Elite 4 content. Adventures: Red Chapter follows the manga adventures of Red. It’s in a redesigned Kanto and has a lot of dialogue. The creator is in the process of updating the entire thing so I’m not sure how long the most current Beta is. Ash Gray follows the anime adventures of Ash. It is very close to the original show.
I don’t think it is complete but is very long. Victory Fire, Resolute, and Mega Power are all made by the same guy. Res is a sort of sequel to VF. None are incredible, but they all have at least one new region and a new story. Also require more grinding than I prefer. Giratina Strikes Back has a new region and story.
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Also has some Fakemon but none are super well done. Story features Samus Aran and Darth Vader though so that’s cool. Vega is a Japanese hack translated to English and features mostly Fakemon. Many are very well done.
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There is a version called Vega Minus that makes the game a bit easier since Vega has some stupidly OP gym leaders and you can’t buy Revives anywhere. Ultra Shiny Gold Sigma is a bit of a divisive hack. It’s basically Gen 2 (Johto then Kanto) but adds in some different story elements. I think the game is super long though. It’s like Johto, then Kanto, then the Orange Islands, and I think the creator is working on adding in Hoenn too. It’s got a lot of bugs though so play at your own risk. Gaia isn’t complete.
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Last time I checked it was up to like 7 gyms. Very high quality though if a bit too hand-holdy at times. There are also GBA enhancement hacks but I can’t speak for what they add:. Gen 1: Red. Gen 2: Crystal Dust or Liquid Crystal. Gen3: Theta Emerald EX and Nameless Fire Red.